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3()(10176025):,1980,,31,1,2(1,621010;2,730060),5,ResearchandApplicationStatusofRadioactiveWasteSolidificationCHEChunxia1,TENGYuancheng1,GUIQiang2(1SichuanProv.KeyLabofAdvancedConstructionMaterial,SouthwestUniversityofScienceandTechnology,Mianyang621010;2PetrochemicalResearchInstituteofLanzhouPetrochemicalCompany,Petrochina,Lanzhou730060)AbstractItisanimportantproblemtodisposeradioactivewastesafelyandefficiently,whichistheguaranteeofhealthyandcontinuousdevelopmentfornuclearindustry.Oneofdevelopmenttrendsistosolidifytheradioactivewasteandthentoburyit.Thispaperanalysesanddiscussedsolidificationtheories,statusofsolidificationresearchandapplication,applicationfield,advantageanddisadvantageofcementsolidification,bitumensolidification,plasticsolidi2fication,glasssolidificationandsynrocsolidificationquitesystematically.Cementsolidification,bitumensolidificationandplasticsolidificationarefittodisposelowandintermediatelevelradioactivewaste.Glasssolidificationandsynrocsolidificationarefittodisposehighlevelradioactivewaste.Keywordsradioactivewaste,cementsolidification,bitumensolidification,plasticsolidification,glasssolid2ification,synrocsolidification0,,,,,,[13],,3:;,;,(ILLW),;(HLW),[47],,,,,,,1,,40ILLW,,ILLW[4],[8,9]:,,,4920062202[10],(1):,;,,,,,;,,,200300m,,,,(ORNL)60Ci,65%,(100400)(1707000MPa),,,[4,11]1:,;,,;[10]:,;1.52,,[10]21960,,60,1984,ILLW,,,,[1214]:,,[10,15]3,,,,,,,[12]2[10]2,:,;(1112),,;[10]:,,,,;;,,32070,,:,,,,[10]:,,[10],,,2070,,,,50%,40%20%50%TBP,40%50%TBP,,,,,,[4],,,,59/,,,[16,17],:,,24,;,,[16],:,;,;42050,,2070HLW30,HLW,HLW[18]:,(9001200),HLW:,,,HLW,ILLW[10],HLW,,PIVER2070,,,,,+,AVMAVHAVW,(PNNL),PAMELA,,,2,,(Saluggia),,(RADON),[19]3HLWHLW:(),,[20]3[10]:,10%30%(wt);[22]:,,,,,,;,;51978Rinwood(Synroc),,HLW,1993,[2225]:,,,,,,,HLW[26],,,[27],,,1m(2050nm)[28,29],,HLW,HLW4,(ANSTO)1987(4[4]),10kg/h,800tHLW,6920062202,1.76MHz60kW,1600[23](CaZrTi2O7)(TiO2)(BaAl2Ti6O16)(CaTiO3)(CaUTi2O7)(CaTiSiO5)(ZrSiO4)(ZrO2)(CePO4)(Ca4-xREE6+x2(SiO4)6-y(PO4)y(O,F)2),HLW[30],,,,H2,TiH2H2,2%(),(HUP)(HIP)(AS)[4,31,32],:;,,,,;HLW,,HLW30%,HLWB45%,HLWB60%;,[21]:,,(),,,,HLW,,HLW,6,ILLW,,,,,,ILLWHLW,HLW,,,,,HLW,,,,HLW,,HLW,HLW1YlvaUggla.Riskandsafetyanalysisinlong2termperspec2tive[J].Futures,2004,(36):5492HamdiEl2Ghonemy,LenWatts,LindaFowler.Treatmentofuncertaintyanddevelopingconceptualmodelsforenviron2mentalriskassessmentsandradioactivewastedisposalsafe2tycases[J].EnvironmentInternational,2005,31(1):893BrodenK,OlssonG.Finaldisposalpossibilitiesofradioac2tivewastecomponentsfromITER[J].FusionEngineeringandDesign,2003,69(4):6954.[M].:,2003.1175KyongWonHan,HeinonenJ,BonneA.Radioactivewastedisposal:globalexperienceandchallenges[J].IaeaBulle2tin,1997,39(1):336StegemannJA,CotePL.Aproposedprotocolforevalua2tionofsolidifiedwastes[J].ScienceofTheTotalEnviron2ment,1996,178(3):1037FerencLToth,Hans2HolgerRogner.Oilandnuclearpow2er:past,present,andfuture[J].EnergyEconomics,2006,28(1):18OlsonRA,TennisPD,BonenD,etal.Earlycontainmentofhigh2alkalinesolutionsimulatinglow2levelradioactivewasteinblendedcement[J].JHazardousMaterials,1997,52(2):2239MichelineMoranville,SihamKamali,EmmanuelGuillon.Physicochemicalequilibriaofcement2basedmaterialsinag2gressiveenvironments2experimentandmodeling[J].CementConcreteResearch,2004,34(9):156910.[M].:,2004.24711GlasserFP,AtkinsM.Cementsinradioactivewastedis2posal[J].MRSBull,1994,19(12):3312.[J].,1998,(32)5:3713HabersbergerovaA,KrejciF,TimulakJ.Solidificationofradioactivewastesbybituminizationtechnology,radiationstabilityofbitumenproducts[J].JadernaEnergie,1986,32(12):44914KenOkada,RifaidMNur,YasuhikoFujii.Theformationofexplosivecompoundsinbitumen/nitratemixtures[J].JHazardousMater,1999,69(3):24515AwwalMA,GuzellaMFR,SilvaTV.Chemicaltreatmentofsimulatedsolutionofevaporatorconcentrateforimmobilizationinbitumen[J].WasteManagement,1996,16(4):25116.[J].,1985,(11):42817NedomaJ.Onacoupledstefan2likeprobleminthermo2visco2plasticrheology[J].JComputationalAppliedMathematics,1997,84(1):45(101)79/6BednorzJZ,MllerKA.ZPhysB,1986,64:1897ChuCW,etal.PhysRevLett,1987,58:9088ZhaoZhongxian,ChenLiquan,etal.KexueTongbao,1987,10:6619JaejunYu,MassiddaS,FreemanAJ.PhysicaC,1988,152:27310BreitzkeH,EreminI,etal.PhysicaC,2004,406:2711MasaruTomita,MasatoMurakamiI.Nature,2003,421:51712,.,1995,9():25713ValladaresLuisDeLosSantos,AngelBustamanteD,etal.PhysicaC,2004,4082410:4414FruthV,PopaM,etal.JEurCeramSoc,2004,24:182715SinhNH.JMagnMagnMater,2003,262:51416TepeM,AvciI,etal.SolidStateCommunications,2004,131:31917YangPeidong,CharlesMLieber.Science,1996,273:183618KummethP,StrullerC.ApplPhysLett,1994,65:130219NagamatsuJ,NakagawaN,Maranaka,etal.Nature,2001,410:6320LorenzB,MengRL,ChuCW.PhysRevB,2001,64:010226421HinksDG,JorgensenJD.PhysicaC,2003,385:9822KnagWN,JungetalCU.PhysRevB,2001,64:010231323JoshiAG,etal.SolStaCom,2001,118:44524FuchsG,etal.SolStaCom,2001,118:49725MullerKH,FuchsG,etal.AlloyComp,2001,322:L1026WangYuxing,TomaszPlackowski,AlainJunod.PhysC,2001,353:17927CucoloAM,BobbaaF,etal.PhysicaA,2004,339:11228RubioBollingerG,SuderowHS.PhysRevLett,2001,86(24
本文标题:放射性废物固化处理的研究及应用现状
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